>> Primary Particulate Matter Emitted from Heavy Fuel and Diesel Oil Combustion in a Typical Container Ship: Characteristics and Toxicity

2018-12-15阅:299

题名:Primary Particulate Matter Emitted from Heavy Fuel and Diesel Oil Combustion in a Typical Container Ship: Characteristics and Toxicity

来源:Environmental Science & Technology

发表年代:2018年

作者:Di Wu, Qing Li, Xiang Ding, Jianfeng Sun, Dan Li, Hongbo Fu, Monique Teich, Xingnan Ye, and Jianmin Chen

Abstract Container ships have been widely recognized as an important emission source within maritime transport. Heavy fuel oil (HFO) and diesel oil  (DO) are the two most commonly used fuels. This study reports the  characteristics and toxicities of particulate matter (PM) emissions from  HFO and DO combustion in a typical container ship. The PM number size  distribution possesses a bimodal structure with peaks at ~20 nm and ~100  nm. The PM2.5 emission factor (EF) are 3.15 ± 0.39 and 0.92 ± 0.02 g/kg  fuel for HFO and DO, respectively. The benzo[a]pyrene equivalent  carcinogenic potency (BaPeq) of 16 polycyclic aromatic hydrocarbons  contained in HFO and DO PM2.5 are approximately 0.81 ± 0.10 and 0.12 ±  0.04 mg/kg fuel, respectively. BaPeq concentration shows an increasing  tendency with decreased PM size. The reactive oxygen species activity  and cytotoxicity of HFO PM2.5 samples are ~2.1 and ~2.5 times higher  than those of DO PM2.5 samples, respectively. These health risks are  both significantly attributed to the BaPeq content in PM2.5 with  correlations of 0.86~0.92. Furthermore, the examined biological effects  are much greater than those of PM2.5 collected in Shanghai. Our results  imply that better fuel quality is important for improving air quality  and reducing health risks.

Primary Particulate Matter Emitted from Heavy Fuel and Diesel Oil Combustion in a Typical Container Ship – Characteristics and Toxicity.pdf